My money is on leak off pipes letting air into the mix or dirty/failing injectors.
I take it that, at no point have you let the tank run to the point where you need more than 60L to fill it. There's the obvious risk of pulling up crud off the bottom of the tank, but also the risk of air getting into the fuel mix and damaging the injector control unit. It's not a given failure considering, when I picked up mine a few years ago I put 70.2 litres into it and it's been fine ever since, it's just not worth risking.
When you're checking the fuel side don't forget the rusty plate under the boot floor that sits above the fuel pump and the state of the hoses attached to it. Depending on how much it's disintegrated it could be dropping muck into the fuel.
Don't think a slipped timing chain is likely, the chain and sprocket are far better meshed than with a cambelt, but I think it's an interference engine, so it would be curtains for some of the valves. If experience is anything to go by, you'd here a horrible metal mashing noise.